江苏大学汽车与交通工程学院,江苏,镇江,212013
网络首发:2018-03-10,
纸质出版:2018
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顾林波, 蔡忆昔, 施蕴曦, 等. 间接低温等离子体对柴油机颗粒物成分及官能团的影响[J]. 西安交通大学学报, 2018,52(3):63-68.
Effect of INTP on the Composition and Functional Groups of PM in Diesel Engine[J]. 2018, 52(3): 63-68.
顾林波, 蔡忆昔, 施蕴曦, 等. 间接低温等离子体对柴油机颗粒物成分及官能团的影响[J]. 西安交通大学学报, 2018,52(3):63-68. DOI: 10.7652/xjtuxb201803009.
Effect of INTP on the Composition and Functional Groups of PM in Diesel Engine[J]. 2018, 52(3): 63-68. DOI: 10.7652/xjtuxb201803009.
为探究间接低温等离子体(INTP)对柴油机颗粒物(PM)成分及官能团的影响
以氧气作为介质阻挡放电式低温等离子体发生器的气源
搭建了INTP技术处理柴油机PM的试验台架
利用热重分析仪、傅里叶红外光谱仪和微克天平探究了低温等离子体对柴油机PM成分、官能团和质量的影响。试验结果表明:INTP处理后PM的成分发生了明显变化
挥发性物质的质量分数下降至48%~71%
固体碳的含量上升至29%~52%; PM的特征温度和表观活化能都有所下降
INTP降低了PM的氧化温度
提高了PM的氧化活性; INTP处理后
PM表面的烷基官能团减少
新生成的含氧官能团和芳香环使PM氧化活性增强; 经过INTP处理后
柴油机PM去除量为7.91~26.732 mg
去除率为40%~80%。
In order to investigate the effect of indirect non-thermal plasma(INTP)on composition and functional groups of diesel particulate matter(PM)
oxygen was used as the gas source of non-thermal plasma reactor with dielectric barrier discharge and a test bench for the treatment of diesel PM by using INTP technology was built up. A thermo-gravimetric analyzer
a Fourier transform infrared spectroscopy and a microgram balance were used to investigate the effects of non-thermal plasma on the composition
functional groups and quality of PM. The results show that the composition of PM changes obviously after the treatment of INTP. The proportion of volatile matter falls to 48%-71%
and solid carbon accounts for an increase to 29%-52%. The characteristic temperatures and apparent activation energy of PM both decrease after INTP
so INTP has the ability to make PM easier to be oxidized at a lower temperature and improve the oxidation activity of PM. After the treatment of INTP
the alkyl functional groups on the PM surface are reduced
and the newly formed oxygen-containing functional groups and aromatic rings enhance the PM oxidation activity. The removal mass and rate of PM is 7.91-26.732 mg and 40%-80% respectively after INTP treatment.
WANG Y, RAJ A, CHUNG S H. A PAH growth mechanism and synergistic effect on PAH formation in counter flow diffusion flames [J]. Combustion and Flame, 2013, 160(9): 1667-1676
黄震, 李新令, 吕田, 等. 燃料特性对柴油机排放颗粒物理化特性影响的研究 [J]. 内燃机学报, 2016, 34(2): 97-104.
HUANG Zhen, LI Xinling, LÜ Tian, et al. Study on post treatment of particulate emissions from diesel engine test [J]. Transactions of CSICE, 2016, 34(2): 97-104.
刘志华, 葛蕴珊, 丁焰, 等. 柴油机和LNG发动机排放颗粒物粒径分布特性研究 [J]. 内燃机学报, 2009, 27(6): 518-522.
LIU Zhihua, GE Yunshan, DING Yan, et al. The size distribution characteristic of PM emitted from diesel engine and LNG engine [J]. Transactions of CSICE, 2009, 27(6): 518-522.
VINOGRADOV J, RIVIN B, SHER E. NOx reduction from compression ignition engines with DC corona discharge: An experimental study [J]. Energy, 2007, 32(3): 174-186.
陈思乐, 许桂敏, 穆海宝, 等. 低温等离子体处理柴油机尾气的研究进展 [J]. 高压电器, 2016, 54(4): 22-29.
CHEN Sile, XU Guimin, MU Haibao, et al. Research progress in treatment of diesel engine exhaust by non-thermal plasmas [J]. High Voltage Apparatus, 2016, 54(4): 22-29.
姚水良, 赵一帆, 张媛, 等. 多层介质阻挡放电处理柴油机尾气颗粒物 [J]. 浙江大学学报(工学版), 2015, 49(1): 157-161.
YAO Shuiliang, ZHAO Yifan, ZHANG Yuan, et al. Treatment of particle material from diesel exhaust using multilayer dielectric barrier discharge [J]. Journal of Zhejiang University(Engineering Science), 2015, 49(1): 157-161.
ANAGHIZI S J, TALEBIZADEH P, RAHIMZADEH H, et al. The configuration effects of electrode on the performance of dielectric barrier discharge reactor for NOx removal [J]. IEEE Transactions on Plasma Science, 2015, 43(6): 1944-1953.
邢世凯, 马朝臣, 马松. 低温等离子体对柴油机排气微粒数量和质量影响的试验研究 [J]. 内燃机工程, 2013, 34(1): 8-12.
XING Shikai, MA Chaochen, MA Song. Experimental study of effects of non-thermal plasma on exhaust PM quantity and mass in diesel engine [J]. Chinese Internal Combustion Engine Engineering, 2013, 34(1): 8-12.
OKUBO M, KUROKI T, KAWASAKI S, et al. Continuous regeneration of ceramic particulate filter in stationary diesel engine by nonthermal-plasma-induced ozone injection [J]. IEEE Transactions on Industry Applications, 2009, 45(5): 1568-1574.
SHI Y, CAI Y, WANG J, et al. Influence of PM size distribution and ingredients on DPF regeneration by non-thermal plasma technology [J]. Plasma Chemistry and Plasma Processing, 2016, 37(2): 1-14.
SHI Y X, CAI Y X, LI X H, et al. Mechanism and method of DPF regeneration by oxygen radical generated by NTP technology [J]. International Journal of Automotive Technology, 2014, 15(6): 871-876.
施蕴曦, 蔡忆昔, 李弘扬, 等. 氧气流量控制策略对低温等离子体技术再生柴油机微粒捕集器的影响 [J]. 西安交通大学学报, 2016, 50(9): 74-79.
SHI Yunxi, CAI Yixi, LI Hongyang, et al. Effect of oxygen flow control strategy on diesel particulate filter regeneration by non-thermal plasma technology [J]. Journal of Xi'an Jiaotong University, 2016, 50(9): 74-79.
何百磊, 宋蔷, 姚强, 等. 钙钛矿型催化剂催化氧化碳黑的活性分析 [J]. 中国电机工程学报, 2007, 27(2): 54-58.
HE Bailei, SONG Qiang, YAO Qiang, et al. Activity analysis of catalytic oxidation of carbon black over various perovskite-type catalysts [J]. Proceeding of the CSEE, 2007, 27(2): 54-58.
李博. 燃料特性对柴油机颗粒物表面官能团及氧化活性影响研究 [D]. 天津: 天津大学, 2013.
梅德清, 赵翔, 王书龙, 等. 柴油机排放颗粒物的热重特性分析 [J]. 农业工程学报, 2013, 29(16): 50-56.
MEI Deqing, ZHAO Xiang, WANG Shulong, et al. Thermogravimetric characteristics analysis of particulate matter of emission of divided diesel [J]. Transactions of the Chinese Society of Agricultural Engineering, 2013, 29(16): 50-56.
孟忠伟, 杨冬, 闫妍, 等. 柴油机尾气颗粒和碳黑颗粒氧化特性的分析比较 [J]. 燃烧科学与技术, 2016, 22(1): 71-76.
MENG Zhongwei, YANG Dong, YAN Yan, et al. Comparison of oxidation characteristic analysis between diesel soot and carbon black [J]. Journal of Combustion Science and Technology, 2016, 22(1): 71-76.
张东明. 柴油机燃烧过程中颗粒物表面官能团变化规律的研究 [D]. 天津: 天津大学, 2009.
郝斌. 不同燃料对柴油机排气颗粒物的影响研究 [D]. 天津: 天津大学, 2014.
SONG J, ALAM M, BOEHMAN A L, et al. Examination of the oxidation behavior of biodiesel soot [J]. Combustion and Flame, 2006, 146(4): 589-604.
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